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Well, I'm a wierdo who processes vocals as musical instruments and often don't pay any attention to lyrics, so I don't literally know all the words to any album - unless you count the Star Wars & Empire Strikes Back soundtracks that have no spoken words. But if you're talking "have listened to the album front to back so much that I could accurately pretend to sing along with every word", I'd easily go with:
Beastie Boys - License to Ill (@moxie; very first album I thought of, too.)
System of a Down - Toxicity
A Tribe Called Quest - Midnight Marauders